Dynamics of the collective modes of an inhomogeneous spin ensemble in a cavity

We study the excitation dynamics of an inhomogeneously broadened spin ensemble coupled to a single cavity mode. The collective excitations of the spin ensemble can be described in terms of generalized spin waves and, in the absence of the cavity, the free evolution of the spin ensemble can be described as a drift in the wave number without dispersion. In this article we show that the dynamics in the presence of coupling to the cavity mode can be described solely by a modified time evolution of the wave numbers. In particular, we show that collective excitations with a well- defined wave number pass without dispersion from negative to positive valued wave numbers without populating the zero wave number spin wave mode. The results are relevant for multi-mode collective quantum memories where qubits are encoded in different spin waves.Comment: Published version. Some small changes and correction

The field inside a random distribution of parallel dipoles

We determine the probability distribution for the field inside a random uniform distribution of electric or magnetic dipoles. For parallel dipoles, simulations and an analytical derivation show that although the average contribution from any spherical shell around the probe position vanishes, the Levy stable distribution of the field is symmetric around a non-vanishing field amplitude. In addition we show how omission of contributions from a small volume around the probe leads to a field distribution with a vanishing mean, which, in the limit of vanishing excluded volume, converges to the shifted distribution.Comment: RevTeX, 4 pages, 3 figures. Submitted to Phys. Rev. Let

Scalable designs for quantum computing with rare-earth-ion-doped crystals

Due to inhomogeneous broadening, the absorption lines of rare-earth-ion dopands in crystals are many order of magnitudes wider than the homogeneous linewidths. Several ways have been proposed to use ions with different inhomogeneous shifts as qubit registers, and to perform gate operations between such registers by means of the static dipole coupling between the ions. In this paper we show that in order to implement high-fidelity quantum gate operations by means of the static dipole interaction, we require the participating ions to be strongly coupled, and that the density of such strongly coupled registers in general scales poorly with register size. Although this is critical to previous proposals which rely on a high density of functional registers, we describe architectures and preparation strategies that will allow scalable quantum computers based on rare-earth-ion doped crystals.Comment: Submitted to Phys. Rev.

Quantum simulation of the hexagonal Kitaev model with trapped ions

We present a detailed study of quantum simulations of coupled spin systems in surface-electrode ion-trap arrays, and illustrate our findings with a proposed implementation of the hexagonal Kitaev model [A. Kitaev, Annals of Physics 321,2 (2006)]. The effective (pseudo)spin interactions making up such quantum simulators are found to be proportional to the dipole-dipole interaction between the trapped ions, and are mediated by motion which can be driven by state-dependent forces. The precise forms of the trapping potentials and the interactions are derived in the presence of a surface electrode and a cover electrode. These results are the starting point to derive an optimized surface-electrode geometry for trapping ions in the desired honeycomb lattice of Kitaev's model, where we design the dipole-dipole interactions in a way that allows for coupling all three bond types of the model simultaneously, without the need for time discretization. Finally we propose a simple wire structure that can be incorporated in a microfabricated chip to generate localized state-dependent forces which drive the couplings prescribed by this particular model; such a wire structure should be adaptable to many other situations.Comment: 24 pages, 7 figures. v2: simplified the derivation of (28) without changing conclusions; minor edits. v3: minor edit

Quantum computing with an electron spin ensemble

We propose to encode a register of quantum bits in different collective electron spin wave excitations in a solid medium. Coupling to spins is enabled by locating them in the vicinity of a superconducting transmission line cavity, and making use of their strong collective coupling to the quantized radiation field. The transformation between different spin waves is achieved by applying gradient magnetic fields across the sample, while a Cooper Pair Box, resonant with the cavity field, may be used to carry out one- and two-qubit gate operations.Comment: Several small corrections and modifications. This version is identical to the version published in Phys. Rev. Let

Transport and Spectroscopic Studies of the Effects of Fullerene Structure on the Efficiency and Lifetime of Polythiophene-based Solar Cells

Time-dependent measurements of both power conversion efficiency and ultraviolet-visible absorption spectroscopy have been observed for solar cell blends containing the polymer poly(3-hexylthiophene-2,5-diyl) (P3HT) with two different functionalized C60 electron acceptor molecules: commercially available [6,6]-phenyl C61 butyric acid methyl ester (PCBM) or [6,6]-phenyl C61 butyric acid octadecyl ester (PCBOD) produced in this laboratory. Efficiency was found to decay with an exponential time dependence, while spectroscopic features show saturating exponential behavior. Time constants extracted from both types of measurements showed reasonable agreement for samples produced from the same blend. In comparison to the PCBM samples, the stability of the PCBOD blends was significantly enhanced, while both absorption and power conversion efficiency were decreased.Comment: manuscript submitted to Solar Energy Materials and Solar Cell

Spectroscopic properties of inhomogeneously broadened spin ensembles in a cavity

In large ensembles of identical atoms or spins, the interaction with a mode of the electromagnetic radiation field concentrates in a single superradiant degree of freedom with a collectively enhanced coupling. Given a controllable inhomogeneous broadening, such ensembles may be used for multi-mode storage of quantum states of the radiation field with applications in quantum communication networks and quantum computers. In this paper we analyze how the width and shape of the inhomogeneous broadening influence the collective enhancement and the dynamics of the cavity-ensemble system with focus on the consequences for the ensemble's applicability for quantum information processing tasks.Comment: 12 pages, 5 figure

Scalable ion traps for quantum information processing

We report on the design, fabrication, and preliminary testing of a 150 zone array built in a `surface-electrode' geometry microfabricated on a single substrate. We demonstrate transport of atomic ions between legs of a `Y'-type junction and measure the in-situ heating rates for the ions. The trap design demonstrates use of a basic component design library that can be quickly assembled to form structures optimized for a particular experiment